Appendix A.
Daily transport and surface deposition of 137Cs
The atmospheric dispersion and deposition of radionuclides released from FNPP1 were generally reproduced by the simulation with the refined source term (Movie A1). Regional-scale atmospheric dispersion and surface deposition of 137Cs during March 2011 were explained as follows. Detailed analysis of local-scale atmospheric dispersion from March 12 to 17 is described in Katata et al. (2012a,b). Supplementary video related to this article can be found at doi: 10.1016/j.jenvrad.2012.05.023.
March 12-14
The radioactive plume discharged from FNPP1 first flowed toward the Pacific Ocean over the early morning to the afternoon on March 12. The high-concentration plume around the hydrogen explosion, which occurred at Unit 1 at 15:30 JST on March 12, flowed in the north-northwest direction from FNPP1 and caused a large amount of dry deposition. An increase in air dose rate was observed at the monitoring post of Minami-soma (shown in Fig. 6a) 4.5 h after the explosion (Fukushima Prefecture, 2011). The plume then flowed in the northenortheast direction and produced a large amount of dry deposition in the northeastern coastal area of Miyagi Prefecture (Figs. 6a and 7a). Air dose rates observed at the nuclear power plant in Onagawa (shown in Fig. 6a) were elevated at 0 JST on March 13 when the plume passed through (Tohoku Electric Power, 2011). Afterwards, the plume was transported mainly towards the ocean by the southwesterly wind until the night of March 14.
March 15
The high-concentration plume started to flow in the south-southwest direction from FNPP1 from late at night on March 14 and caused a large amount of dry deposition along the southeastern coastal area of Fukushima Prefecture and the northeastern area of Ibaraki Prefecture on the morning of March 15 (Figs. 6b and 7b). The plume successively dispersed and caused dry deposition in Tokyo, Saitama, and Kanagawa Prefectures, although the quantity was smaller than in the above regions. From the afternoon of March 15, precipitation was observed broadly across eastern Japan (Fig. 7c), due to a low pressure system passing through Honshu. The calculated plume encountered the rain band over the areas of Niigata, Gunma, Tochigi, and Fukushima Prefectures, and this caused a large amount of wet deposition in the afternoon (Figs. 6c and 7c). Then, the plume changed its direction clockwise to the northwest of FNPP1, and passed through Miyagi, Yamagata, and Iwate Prefectures during the evening and into the night. In Fukushima Prefecture, the high-concentration plume, due to the major release from FNPP1 in the afternoon, caused significant dry and wet deposition in the area northwest of FNPP1 (Katata et al., 2012a,b).
Although a large amount of surface deposition of 137Cs was observed by airborne monitoring in the north of Tochigi and Gunma Prefectures (MEXT, 2011d), in the calculation, it was mainly seen in the south of Niigata Prefecture and the west of Fukushima Prefecture (Fig. 8b). Because no comparable amount of surface deposition was calculated on other days in the north of Tochigi and Gunma Prefectures, the deposition on March 15 has the largest contribution to the total deposition for the area. From the observed precipitation and air dose rate (MEXT, 2011a; Tochigi Prefecture, 2011), the discrepancy is due to the high-concentration plume passing through Tochigi and Gunma Prefectures before the occurrence of precipitation in the area. In Tochigi Prefecture, additional surface deposition of 137Cs contained in fog or cloud observed at
Okunikko (shown in Fig. 7c) may also contribute to the observed surface deposition.
In the calculation, a significant amount of wet deposition also appeared in the area from the north of the central part of Fukushima Prefecture, via Miyagi Prefecture, to the south of Iwate Prefecture, which was not the case from ground-level and airborne monitoring (MEXT, 2011a,d; Miyagi Prefecture, 2011). Considering that, in the calculation, the principal part of the plume was transported above the clouds (not shown in figures), a possible cause of the discrepancy between calculation and observation is the overestimation of wet deposition in the upper air in the model.
March 16-19
The plume was calculated to have flowed mostly toward the ocean, due to the wind fluctuating from westerly to northwesterly from March 16 to 19. In the observations, however, air dose rate monitoring in the southeast of Fukushima Prefecture and in the east of Ibaraki Prefecture (Fukushima Prefecture, 2011; Ibaraki Prefecture, 2011; KEK, 2011; MEXT, 2011a) during the morning of March 16 suggests that the plume flowed over Ibaraki Prefecture and produced a lot of dry and wet deposition on that morning. The model could not reproduce the above surface deposition because of errors in the calculated wind direction.
March 20
The plume, which flowed to the east of FNPP1, started to turn clockwise before dawn on March 20. The plume passed over the Kanto region in the morning, and then changed its direction to the northwest of FNPP1 in the afternoon. The plume flowed to the west of Miyagi Prefecture, to the east of Yamagata Prefecture, and to the south of Iwate Prefecture. A large amount of wet deposition was produced in the area, due to precipitation in the evening (Figs. 6d and 7d). The plume started to flow to the south of FNPP1 again late at night.
March 21
The plume flowed into Ibaraki Prefecture via the ocean on the morning of March 21, then dispersed over the Kanto region and caused a large amount of wet deposition in Ibaraki, Chiba, Saitama, Tokyo, and Kanagawa Prefectures due to precipitation from the morning (Figs. 6e and 7e). Surface depositions were overestimated at the sampling sites of Kofu and Omaezaki (Nos. 17 and 18, Fig. 1) because of the overestimation of daily precipitation.
March 22
The plume released from FNPP1 on March 22 dispersed mainly in Fukushima and Tochigi Prefectures, and caused wet deposition in the east of Fukushima Prefecture due to precipitation from the night (Figs. 6f and 7f). Meanwhile, the radionuclides released on March 21 remained stagnant in the Kanto region and were deposited by precipitation on March 22.
March 23-24
From the early morning on March 23, the plume was transported along the seaside of Ibaraki and Chiba Prefectures, due to the wind fluctuating from northerly to northwesterly. It flowed into the southeastern part of the Kanto region from the afternoon and produced wet deposition from the evening until late at night (Figs. 6g and 7g). The plume was mostly transported toward the ocean from the morning of March 24 to the morning of March 25.
March 25-29
From the afternoon to the night of March 25, the plume was transported by the southeasterly wind in the northwest direction from FNPP1, and caused wet deposition mainly in Fukushima Prefecture and in the south of Yamagata and Miyagi Prefectures (Figs. 6h and 7h). Then, the plume changed its direction anticlockwise from northwest to southeast on the morning of March 26. The plume continuously flowed toward the ocean from the morning of March 26 to March 29.
March 30-31
The plume turned clockwise from the east to the southwest of FNPP1 and flowed into the Kanto region on the morning of March 30, and caused wet deposition mainly in Tochigi and Ibaraki Prefectures during the afternoon (Figs. 6i and 7i). The plume from FNPP1 then flowed in the northwest direction from FNPP1 from the afternoon until the night. On March 31, the plume mainly flowed toward the ocean.